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Santorini Greek Islands Honeymoon in Greece Santorini is the number one destination in the Greek Islands for a honeymoon, and for good reason. Santorini is one of the most romantic places on earth. Pam and Armie visited Santorini on their Greece honeymoon. They based themselves in Imerovigli, just outside of Thira, to explore the rest of the beautiful island. There is a working archaeological excavation at the ruins of Akrotiri, linked with the Atlantis Myth, and Oia is famous for it's sunset.